English
聯系我們
網站地圖
郵箱
舊版回顧



中國科大在單分子電致上轉換發光的實驗觀察與機理研究中取得進展

文章來源:中國科學技術大學   發布時間:2019-05-10  【字號:     】  

  最近,中國科學技術大學單分子科學團隊的董振超研究小組,通過掃描隧道顯微鏡(STM)誘導單分子電致發光技術,首次清晰地展示了單個分子在電激勵下的上轉化發光行為,并通過與深圳大學教授李曉光等合作,從理論上揭示了其微觀機制。國際物理學術期刊《物理評論快報》于53日在線發表了這項成果。

  上轉換發光通常指材料吸收低能光子但發出高能光子的反斯托克斯過程,這一現象在激光信息技術、紅外探測、生物醫學等領域有巨大的應用前景。電激勵下的上轉化發光過程中,有機分子吸收由STM注入的低能電子,并在其弛豫過程中發射出高能光子。這一過程涉及分子電子能態、分子間以及分子與周圍環境間的相互作用,深入理解這些相互競爭與制約的微觀過程,對其在有機光電轉換器件、光催化和光合成等方面的應用有著至關重要的意義。

    中國科大單分子科學團隊長期致力于發展將STM高空間分辨表征與光學技術高靈敏探測相結合的技術,特別是通過巧妙調控隧道結納腔等離激元的寬頻、局域與增強特性,拓展了測量極限,為在單分子水平上觀測和調控分子的光電行為提供了有力手段。他們利用高度局域化的隧穿電子作為激發源,研究了氯化鈉脫耦合層表面上的單個酞菁分子的電致熒光,不僅發現了反常的電致上轉換發光現象,還清晰地展示了分子發光強度的三個不同偏壓區域。尤其值得指出的是,該工作在單分子水平上觀測到電致上轉換發光現象,有力排除了此前對這類體系中上轉換機制的一些猜測,同時不同偏壓區域的觀測也為分析和理解上轉換機制提供了豐富的數據。以此為基礎的理論分析進一步表明,兩種不同的分子激發機制——非彈性電子散射和載流子注入——之間的微妙競爭導致了不同偏壓區域不同的發光現象。基于對上述兩種激發機制以及對系統其它潛在激發態的定量分析,研究團隊首次提出了以自旋三重態作為中間過渡態,同時結合非彈性電子散射和載流子注入兩種激發過程的單分子上轉換發光機制。

  陳功與駱陽為這篇文章的共同第一作者。該系列研究工作得到基金委、科技部、中科院、教育部、安徽省等的支持。

  論文鏈接

 

  圖注:(a) STM誘導單分子電致發光的實驗構型示意圖;(b) 三種不同偏壓下單分子電致發光光譜,展示了單分子的上轉換發光現象;(c) 單分子電致發光強度的偏壓依賴關系。




(責任編輯:葉瑞優)

附件:

專題推薦

相關新聞


© 1996 - 中國科學院 版權所有 京ICP備05002857號  京公網安備110402500047號  聯系我們

地址:北京市三里河路52號 郵編:100864

腾讯彩票www.tx65.com www.066504.com | www.69.me | 333144.com | www.2147.xyz | www.9045.loan | www.3040.vip | www.552344.com | 973340.com | 701084.com | www.eh03.com | www.166850.com | 223086.com | www.985.online | www.197651.com | www.514490.com | www.547685.com | www.559252.com | www.775553.cc | www.560359.com | www.444923.com | www.509383.com | www.608974.com | 697753.com | www.27fr.com | www.2017.vip | www.56806.com | www.195631.com | www.751668.com | www.9261.biz | www.052829.com | www.265795.com | www.660700.com | 023890.com | 218163.com | 彩82www.c9223.com | www.79iy.com | www.90sm.com | www.127994.com | 066543.com | www.lw77.com | www.108360.com | www.200587.com | www.297137.com | www.090802.com | www.324644.com | www.491069.com | www.944011.com | 975114.com | 667028.com | www.iz42.com | www.3812.net | www.89773.cc | www.168381.com | www.713910.com | www.906936.com | 063528.com | www.552772.com | 004720.com | www.gm33.cc | www.59oi.com | www.453515.com | www.47au.com | www.878508.com | www.98kt.com | www.302850.com | www.8432.vip | www.31ff.com | www.2210.org | www.329261.com | www.815955.com | 128038.com | 951321.com | www.kd40.com | www.68dh.cc | www.90851.com | www.581448.com | 491208.com | 234144.com | 961483.com | 128043.com | 954587.com | www.07za.com | www.803833.com | www.107011.com | www.18dn.com | www.817556.com | www.181762.com | www.595824.com | www.618259.com | www.847048.com | 945038.com | 554012.com | www.0588.cn | www.81ju.com | www.5789.com | www.85228.cc | www.182338.com | www.682071.com | www.nz06.com | www.zn73.com | www.742985.com | www.390908.com | www.1822.biz | www.972864.com | www.191815.com | 大赢家彩票网www.54400g.com | www.928430.com | www.065881.com | www.21nw.com | www.568729.com | www.608733.com | www.698306.com | www.659423.com | www.712277.com | www.026654.com | www.444258.com | www.376165.com | www.936309.com | www.705404.com | 911784.com | www.1697.cm | www.47044.com | www.731428.com | www.731951.com | 汇发彩票www.hf5882.com | www.606898.com | www.26694.com | 964763.com | www.397013.com | www.69695.cc | 953225.com | www.720234.com | www.13814.com | www.306891.com | www.284129.com | www.pa3.cc | www.kt23.com | www.0860.cm | www.405449.com | www.619929.com | www.967583.com | 幸运彩票www.339189.com | 7581.biz | 787494.com | 149898.com | www.uc17.com | 853937.com | www.eo39.com | www.72924.com | www.024169.com | www.107956.com | www.25zs.com | 304969.com | www.87314.com | www.916234.com | www.5432.cc | www.001678.com | www.68213.cc | www.739372.com | 254861.com | www.029232.com | www.815190.com | 483577.com | www.ly29.com | www.7953.cc | www.150786.com | www.381562.com | www.827679.com | www.ag88988.com | www.005436.com | www.745699.com | 博友彩www.219553.com | www.gi10.com | www.181971.com | www.513111.com | www.854692.com | www.ba1.com | 中国福利彩票www.34788u.com | 大赢家彩票平台www.760320.com | 126934.com | 932901.com | www.0678.in | www.112925.com | www.915342.com | 192285.com | 500彩票www.330297.com | www.tw8.com | www.66xv.com | www.130418.com | www.291417.com | www.378405.com | 423081.com | www.051513.com | www.11867.com | www.14934.com | www.217086.com | www.116874.com | www.166028.com | www.177039.com | www.115062.com | www.177643.com | www.620234.com | www.878116.com | 175389.com | www.ec1.com | www.981169.com | www.881694.com | 949031.com | www.990738.com | www.870362.com | www.985478.com | www.718635.com | www.971093.com | www.993937.com | www.411836.com | www.89kz.com | 673747.com | www.936073.com | www.187268.com | www.111980.com | www.019370.com | 014422.com | www.576671.com | www.873412.com | www.366011.com | www.511095.com | www.475660.com | www.960247.com | www.pz10.com | www.62889.com | kj80.com--kj80.com | 554331.com | www.29du.com | www.80yu.com | www.9083.pw | www.393707.com | www.34169.com | www.611551.com | www.qt74.com | 384817.com | 085775.com | www.972634.com | 177075.com | www.xw71.com | www.654631.com | www.854508.com | www.937434.com | www.920161.com | 万达彩票www.616383.com | www.vz89.com | www.53318.cc | www.393907.com | www.753260.com | 970423.com | www.403699.com | www.677196.com | www.747403.com | www.3690.hk | www.761067.com | www.901901.com | www.776715.com | 524331.com | www.160739.com | 凤凰彩票www.5091c.com | www.58153.com | www.164242.com | www.323968.com | www.372729.com | www.666139.com | 356493.com | www.916679.com | www.802966.com | www.839622.com | 319515.com | www.550328.com | www.4722.vip | www.698991.com | www.881638.com | www.0317.website | www.25hl.com | www.019866.com | www.065813.com | www.301365.com | www.846813.com | www.768167.com | www.866905.com | www.845926.com | www.75xb.com | www.502867.com | www.954227.com | www.970117.com | www.893722.com | 117944.com | 668530.com | 129344.com | 249099.com | www.817749.com | www.39zs.com | 福彩天下www.fcff4.com | 幸运彩票www.112070.com | www.6567.vip | www.285115.com | 038057.com | 924311.com | 福利彩票www.99677b.com | 951541.com | 720059.com | www.953104.com | www.137678.com | www.769520.com | 网易彩票www.089wy.com | www.494153.com | www.4478.com | www.82412.com | www.003621.com | www.69382.com | www.609392.com | 810892.com | 89970.com | www.397577.com | 922604.com | www.991406.com | www.875417.com | 875638.com | 707713.com | 984262.com | 358196.com | www.1510.site | www.au59.com | www.267785.com | www.153545.com | www.705945.com | www.813528.com | www.811323.com | www.852695.com | www.839320.com | 858034.com | 885388.com | www.p33.me | www.c34.org | www.8430.com | www.01230.cc | www.53115.com | www.219159.com | www.287522.com | www.659965.com | www.747775.com | www.560432.com | www.703044.com | www.8628.in | 00ow.com | www.411665.com | 彩宝www.911888a.com | www.174598.com | www.55869.com | www.609899.com | 620791.com | www.cr52.com | www.4825.xyz | www.2960.vip | www.19139.com | www.276577.com | www.449225.com | 890030.com--890070.com | www.7169.org | www.lx47.com | 025428.com | 82244.com | 639405.com | 963454.com | www.915683.com | www.247029.com | www.296177.com | www.032878.com | 388447.com | 533549.com | www.eb98.com | www.366999.com | www.663727.com | www.150697.com | www.889370.com | www.787771.com | PK彩票www.www.23040.com | www.989926.com | www.pt92.com | www.wz34.com | www.062681.com | www.221.me | www.dw3.cc | www.zl77.cc | 13dy.cc | 499887.com | 026934.com | www.679614.com | www.991586.com | www.898342.com | 791354.com | www.968048.com | www.060657.com | 273544.com | www.507042.com | www.2036.cn | 007419.com | www.440560.com | www.175582.com | www.lj.com | www.654547.com | www.6539.top | www.1775.xyz | www.076888.cc | www.256955.com | www.163109.com | www.398012.com | www.974103.com | www.828159.com | www.852879.com | www.920398.com | www.748129.com | 096865.com | www.29230.com | www.01788.cc | www.19974.com | www.12363.com | www.083058.com | www.801763.com | www.785985.com | 212071.com | 358775.com | 739976.com | www.138555.com | www.977316.com | www.798411.com | www.727355.cc | www.649286.com | www.966775.com | 46008.com | www.982404.com | 260690.com | www.tp02.com | www.5301.wang | www.fb05.com | www.78gk.cc | www.881024.com | www.496304.com | www.737009.com | 117766.com | www.2085.vip | www.083760.com | www.850402.com | 58591.com | www.502713.com | www.59674.com | 4632.biz | 027032.com | www.983198.com | www.897828.com | www.728797.com | www.500926.com | www.689925.com | 008704.com | 021096.com | 120893.com | www.453069.com | www.8510.cm | 975248.com | 003584.com | 8k彩票www.803402.com | www.z85.top | www.i53.com | www.12ae.com | www.nm13.com | www.6ku.com | www.267586.com | www.585857.com | 071917.com | 137245.com | 358103.com | www.949756.com | 大富豪www.297277.com | 026043.com | www.791696.com | www.886653.com | www.152222.com | 新淘彩www.715777a.com | 187510.com | www.874693.com | www.801528.com | www.567794.com | 960154.com | yq43.com | www.828772.com | www.560181.com | 68481.com | 731412.com | 919362.com | www.863091.com | 771206.com | 355141.com | www.785065.com | www.773256.com | www.645444.com | www.768739.com | www.572727.com | www.065384.com | www.024004.com | www.9vf.com | www.13085.com | 805657.com | www.341310.com | www.139767.com | www.862811.com | www.958194.com | www.835848.com | www.360311.com | www.572207.com | www.789746.com | www.796062.com | www.930979.com | www.697676.com | www.300652.com | www.162435.com | 6361.biz | www.816011.com | www.512557.com | www.149066.com | www.917128.com | www.807237.com | www.650200.com | www.933192.com | www.784422.com | www.624546.com | www.888599.cc | www.33187.cc | www.96929.cc | www.74pz.com | www.40ec.com | www.3105.com | www.mb33.com | wz85.cc | 256591.com | www.fn7.com | 035303.com | 559623.com | 502050.com | 122865.com | 338024.com | www.864037.com | CP701www.544aa.cc | www.502613.com | www.99jk.com | www.me33.com | www.bp31.com | www.pj46.cc | www.16yh.com | www.cb89.com | www.574440.com | www.6pn.com | 华彩www.71399q.com | 547660.com | 136167.com | www.922783.com | www.599251.com | www.510211.com | www.686699.com | www.273551.com | www.894465.com | www.607531.com | www.t90.top | www.ct2.com | 99彩票www.608986.com | www.5033.biz | www.u77.cc | www.ry24.com | 500彩票www.50064s.com | www.151674.com | www.727841.com | 964092.com | www.99234.cc | www.68nr.com | www.v96.net | www.u88.com | www.hv51.com | www.ln45.com | www.n21.com | 274581.com | 706389.com | 027825.com | www.956946.com | www.3452.com | www.54qk.com | www.15cr.com | www.865686.com | 692503.com | 287661.com | www.lf34.com | 502386.com | www.653965.com | www.352716.com | www.396931.com | www.971840.com | www.922776.com | 126066.com | www.610281.com | www.436036.com | www.127168.cc | www.28593.com | www.979320.com | 493955.com | 629963.com | www.318105.com | www.761947.com | www.385018.com | www.502680.com | www.326563.com | www.306897.com | www.825708.com | www.490104.com | www.119412.com | www.14hk.com | www.122147.com | www.30891.com | 14678.com | 254826.com | 984095.com | 227186.com | 668415.com | 943434.com | www.774028.com | www.78028.cc | www.933171.com | www.850081.com | www.610085.com | www.ee78.com | o78.cc | www.949885.com | www.787011.com | www.771946.com | www.808282.com | www.748244.com | 2334.com | 579471.com | www.980065.com | www.760927.com | www.319423.com | www.283666.cc | www.199530.com | www.657021.com | 254182.com | 076717.com | 062868.com | www.169444.com | www.57944.cc | www.735459.com | www.563281.com | www.196781.com | www.300675.com | www.200509.com | www.502270.com | www.000745.com | 彩82www.c9331.com | 397302.com | www.815922.com | www.484649.com | www.105105.cc | www.246172.com | www.087093.com | www.032372.com | www.9012.org | www.3350.cn | www.672.date | www.44243.com | www.tu47.com | www.44ej.com | 523456.cc | 967492.com | www.5442.cc | www.s90.com | 639224.com | 3314.biz | www.626881.com | www.053959.com | www.81616.com | www.172721.com | 758105.com | www.34126.com | 657454.com | 021056.com | 183917.com | 949283.com | www.964064.com | www.786995.com | www.670991.com | www.609011.com | 578021.com | www.5728.online | www.652082.com | 657649.com | 979254.com | www.2pf.cc | www.207.cm | www.4287.vip | www.01094.com | www.w40.top | 441707.com | www.58604.com | www.65583.cc | www.019143.com | www.304153.com | www.uj65.com | www.248978.com | www.191795.com | www.52565.com | www.85ws.com | www.026677.com | www.1788.live | www.15sj.com | 691102.com | 55世纪www.57pk.cc | 497319.com | www.831558.com | www.te30.com | www.nk30.com | www.203.org | 中国福利彩票www.33588n.com | www.553722.com | 881243.com--pjc55.com | 14500.cc | www.15980.com | www.xi95.com | 530526.com | www.943500.com | da43.com | www.826755.com | 99828.com | 027089.com | www.15368.com | www.90la.com | www.07745.com | www.698403.com | www.505997.com | www.891306.com | 500彩票www.701574.com | www.uh46.com | www.oc45.com | www.2667.in | www.hq45.com | www.6jx.cc | www.9701.com | www.165932.com | www.197902.com | www.63938.com | www.281488.com | 030222.com | 如意彩票www.215889.com | www.099719.com | 401620.com | www.610654.com | 588409.com | 671480.com | 快彩在线www.2632c.com | 061043.com | www.174.bid | www.64891.com | www.025440.com | www.699335.com | www.891772.com | www.57122.cc | www.029137.com | www.101898.com | www.299734.com | www.723952.com | 403665.com | www.793777.cc | www.71zc.com | www.zk67.com | www.81vl.com | www.9510.wang | www.na45.com | 560082.com | www.596041.com | www.529004.com | www.927379.com | www.338762.com | 984807.com | www.67746.com | www.349552.com | www.357070.com | www.275708.com | www.416505.com | www.5214.wang | www.97187.com | www.12277.cc | www.732186.com | 688965.com | www.vp10.com | www.175765.com | www.479409.com | www.086227.com | www.7269.com | www.591867.com | www.012089.com | www.8309.vip | ji05.com | www.941198.com | www.330252.com | www.sr09.com | www.5612.biz | www.159372.com | www.071335.com | www.11256.com | www.21552.com | www.132314.com | www.179757.com | www.87892.cc | 虹彩集团www.hcjt7.com | 034943.com | www.006941.cc | www.8737.net | www.9040.top | www.3532.com | www.086609.com | www.37395.cc | www.170395.com | www.758873.com | www.181799.com | 大众彩票www.925887.com | www.532937.com | www.025206.com | www.157611.com | 412073.com | 708826.com | www.281753.com | 网易彩票www.26163p.com | www.532053.com | www.671660.com | www.60ji.com | 719591.com | www.871123.com | 567479.com | www.293139.com | www.kz89.com | www.cp3.net | www.ql34.com | www.16iw.com | www.667388.com | www.198571.com | www.096627.com | www.100246.com | www.862847.com | www.573293.com | 855615.com | www.1859.wang | 719835.com | www.800652.com | www.ua9.cc | www.106845.com | www.344422.com | www.154.cm | www.092291.com | www.2365.cm | 858453.com | www.825380.com | www.3676.biz | www.1932.vip | www.56705.cc | www.02144.cc | www.079042.com | www.69900.cc | www.103938.com | www.556415.com | www.cai849.com | www.627598.com | www.018847.com | www.950639.com | www.964434.com | www.731605.com | www.0295.net | www.781.me | www.202272.com | www.088828.com | www.42500.cc | www.xs84.cc | www.kp52.com | www.713863.com | www.84xd.com | www.560654.com | www.907269.com | www.611790.com | www.889906.com | 836488.com | www.761.website | www.5wx.com | 611469.com | www.480200.com | 089038.com | www.758302.com | www.8619.in | 137029.com | www.361628.com | www.05530.com | 655008.com | www.547702.com | www.0262.xyz | 159988.com | www.331413.com | www.75320.com | 967349.com | www.85618.com | www.687013.com | www.kj28.com | www.hm49.com | www.630039.com | www.302141.com | www.659119.com | 782616.com | www.tu13.com | 118680.com | 285963.com | www.339342.com | www.383201.com | www.033513.com | www.250358.com | 026492.com | www.965649.com | www.801204.com | www.633376.com | www.mg63.com | www.364003.com | www.400738.com | 947831.com | 262891.com | www.79wn.com | www.uw48.com | www.550401.com | 838399.com | www.33503.com | 博友彩www.941194.com | www.141909.com | www.989944.com | www.802622.com | www.543247.com | www.275186.com | www.003788.com | www.395296.com | 091036.com | 338451.com | www.nm62.com | www.036212.com | 731415.com | 981243.com | www.993646.com | www.669911.com | 533686.com | VIP彩票www.898953.com | www.754955.com | www.921587.com | www.252432.com | www.029873.com | www.7eq.com | 640034.com | www.339414.com | www.796068.com | www.186.in | www.195213.com | 294873.com | 129759.com | www.869070.com | www.919655.com | www.620581.com | 052751.com | 爱彩乐www.652918.com | www.382144.com | www.214844.com | www.72262.cc | 788189.com | www.799809.com | www.807207.com | www.iz88.com | www.i81.net | www.yk08.com | 33068.com | www.764446.com | www.311757.com | www.268716.com | www.6440.com | 亿彩彩票www.yi765.com | 058588.com | www.622446.com | www.605888.com | 3520.biz | www.657.in | www.497276.com | www.467435.com | 凤凰彩票网www.303766.com | www.701584.com | www.1985.cc | www.893034.com | www.15635.cc | www.521689.com | www.111923.com | www.676579.com | 033892.com | www.848608.com | www.678516.com | www.370423.com | www.433876.com | www.131980.com | www.365973.cc | www.682892.com | www.571411.com | 751614.com | www.va08.com | 499151.com | www.379121.com | www.39663.cc | 638535.com | www.080984.com | 50855.com | www.71481.com | www.111935.com | www.524155.com | 576417.com | www.951305.com | www.266933.com | 皮皮彩www.103380.com | www.547361.com | www.ie49.com | www.mr57.com | www.930895.com | www.38527.cc | www.0069.top | 30ec.com | www.113774.com | cp9858.com | www.217419.com | www.788335.com | www.365977.com | www.680215.com | www.670991.com | www.255611.com | www.875286.com | 840711.com | www.6he.com | 851584.com | 659761.com | www.300063.cc | www.lm55.cc | www.071665.com | www.7776.net | www.5bq.com | www.698955.com | www.73zg.com | www.621223.com | www.336980.com | 189222.com | www.247557.com | 579418.com | www.cp3686.com | 329701.com | 55sb.com | www.971601.com | www.654102.com | www.437898.com | www.151364.com | www.665653.com | www.925708.com | 231249.com | 195776.com | www.fp86.com | www.559775.com | www.2720.com | www.88323.com | 334204.com | www.436323.com | 天天彩票www.1035w.com | www.573223.com | www.140810.com | 545379.com | www.484820.cc | www.im66.com | 971539.com | www.659070.com | 750752.com | www.981369.com | www.639401.com | 821257.com | 918115.com | www.882480.com | www.uw10.com | 067899.com | www.896860.com | www.635553.com | cai8181.com | www.187378.com | www.1228.pw | www.38ib.com | www.1661.vip | www.0779.bid | www.169393.com | www.883981.com | www.39931.cc | www.51rz.cc | 821749.com | www.857672.com | www.958438.com | 801828.com | 6474.cc | www.437868.com | www.1479.vip | www.706272.com | www.336707.com | www.9973.pw | www.sn45.com | 274774.com | 386033.com | 891466.com | www.975424.com | 557546.com | www.888278.com | 717377.com | www.729379.com | www.595290.com | www.262636.com | www.70236.com | www.3761.biz | www.29mo.com | www.165875.com | www.919862.com | www.899783.com | www.9139.space | 152932.com | www.324368.com | www.00310.com | 128646.com | www.243366.com | www.1358.vip | www.3938.me | www.733899.com | www.0048.cm | www.g29.club | www.513935.com | www.22861.cc | www.806899.com | www.848574.com | www.391589.com | www.31ij.com | 026214.com | 466928.com | www.674705.com | www.625022.com | 739470.com | www.926145.com | www.431985.com | 986683.com | www.787498.com | 111493.com | 072055.com | www.1179.in | 801993.com | www.113589.com | www.5520.biz | www.234132.com | www.70789.com | www.kh88.cc | www.mt20.cc | 吉利彩票www.80075t.com | www.7783.cc | www.128609.com | 大赢家彩票平台www.226105.com | www.470299.com | www.4467.net | 172361.com | www.6ku.com | www.913797.com | www.8810.cc | www.38959.cc | www.788391.com | www.rx29.com | xz07.com | 500彩票网www.61655w.com | www.rs11.com | www.781142.com | 趣彩网www.qucp7.com | 052521.com | www.832979.com | www.981980.com | 尊彩www.083025.com | 202691.com | 8849.biz | www.693687.com | www.842916.com | www.764382.com | www.cp7553.com | 125390.com | 365675.cc | www.059157.com | www.ip00.com | www.818734.com | www.058930.com | 31553.com | www.326506.com | www.725663.com | 205017.com | www.233838.com | www.222754.com | www.739475.com | 898631.com | www.502613.com | www.257137.com | 877386.com | www.810363.com | www.137085.com | www.oo8.cc | www.179106.com | www.795664.com | www.113266.com | www.81998.com | www.097.net | www.94lg.com | www.bc1.cc | www.4963.biz | www.518942.com | www.585587.com | www.813740.com | www.691261.com | www.747625.com | www.337830.com | www.110455.com | www.44734.com | www.284.tv | www.tw65.com | www.9774.org | www.810343.com | 体彩网www.3890b.com | 982661.com | www.951706.com | www.568752.com | www.446418.com | www.529482.com | www.756233.com | www.697020.com | www.662638.com | www.91658.com | www.b04.top | 584513.com | www.654477.com | 326883.com | 129273.com | www.840923.com | www.763058.com | 937.cc | www.023610.com | 48208.com | www.188283.com | www.140047.com | www.137546.com | www.48by.com | www.617626.com | 326552.com | www.840019.com | www.557560.com | www.695283.com | www.209206.com | www.48103.com | www.po70.com | 048180.com | www.918004.com | www.8579.top | www.726755.com | www.83wq.com | www.560098.com | www.739454.com | www.86zl.com | www.458571.com | www.283925.com | www.413562.com | www.694786.com | www.26dy.com | www.840864.com | www.298112.com | 500彩票www.50064w.com | www.315785.com | 凤凰彩票www.88266c.com | www.615992.com | www.954767.com | www.677549.com | www.155920.com | www.503844.com | www.291135.com | www.515652.com | www.593815.com | www.962042.cc | www.9729.pw | 708022.com--708022.com | www.066082.com | www.85wx.com | 379736.com | 971214.com | 539716.com | www.823635.com | 358427.com | www.404055.com | www.61cy.com | www.596828.cc | www.070400.com | 160673.com | www.224011.com | www.735753.com | 503253.com | www.bs57.com | www.398346.com | www.zz87.com | 684896.com | www.103143.com | www.984600.com | www.300644.com | 001037.com | www.836710.com | www.341536.com | www.659.in | www.95qm.com | 205022.com--502755.com | 646123.com | www.396727.com | www.265716.com | www.14fv.com | www.356687.com | www.39233.com | www.84418.com | www.55em.com | 793138.com | www.739242.com | 064077.com | www.024195.com | 083757.com | www.77173.cc | www.mc77.com | www.837703.com | www.097932.com | www.983866.cc | www.9586.org | www.6206.vip | www.351532.com | www.9751.xyz | www.193612.com | www.61313.com | www.33410.com | www.tf15.com | 139642.com | www.734600.com | www.275286.com | www.084658.com | 7078.biz | www.228312.com | 552031.com | yn46.com | www.39972.cc | 087801.com | www.471127.com | www.011135.com | www.34400.cc | www.29gr.com | www.mv3.com | www.af40.com | www.967104.com | www.779710.com | www.790148.com | www.327601.com | www.20332.com | www.235656.com | 979014.com | www.071619.com | www.975226.com | www.36076.com | www.2552.top | www.762577.com | www.6109.vip | www.850208.com | www.05018.com | www.700267.com | www.670474.com | www.856202.com | www.37249.com | www.7211.com | 588163.com | www.800113.cc | www.985501.com | www.596949.com | www.332319.com | 659441.com | www.194094.com | 052048.com | 500彩票www.50024l.com | www.715058.com | www.07by.com | www.630236.com | www.1704.cn | www.698482.com | www.2344.vip | www.774645.com | www.26gi.com | www.496990.com | 云博彩票www.64422.cc | www.889.gg | www.848113.com | www.603042.com | www.gb60.com | www.104717.com | www.6153.pw | www.30310.com | 55世纪www.202115.com | 500彩票www.50080e.com | www.500899.co | www.312726.com | www.20968.com | www.056967.com | www.522284.com | www.ma2.cc | www.211685.com | www.7216.biz | www.28959.cc | www.83ce.com | 500彩票网www.61655t.com | www.85586.cc | www.35kh.com | www.mb92.com | www.053198.com | www.6179.pw | 654712.com | 619757.com | www.uz46.com | 151590.com | www.966397.com | www.948140.com | www.385605.com | 77437.com | www.905568.com | www.374918.com | www.984717.com | www.006436.com | 166721.com | www.cu99.com | 779581.com | 011993.com | www.967075.com | www.6518.vip | 87ay.com | www.23468.com | www.812051.com | www.20wb.com | www.110261.com | www.32580.com | www.fc41.com | www.6130.cm | 大赢家彩票平台www.503662.com | www.19je.com | dd00.cc | www.536544.com | www.319252.com | 126340.com | www.167726.com | www.956143.com | www.539403.com | www.129534.com | www.168656.com | 340540.com | www.731149.com | www.026264.com | 341368.com | 348103.com | 274527.com | www.752885.com | www.17og.com | www.cp5628.com | 06sd.com | www.74vz.com | 166347.com | 44255.com | 500彩票www.574577.com | www.559121.com | www.om96.com | www.76es.com | www.6274.vip | 701391.com | www.684258.com | www.199010.com | www.209802.com | www.xw39.com | www.8308.hk | www.073145.com | www.731648.com | www.821883.com | www.334200.cc | www.100234.com | www.9909.me | 550994.com | www.913726.com | www.345559.cc | www.4711.biz | www.353350.com | 633342.com | www.612583.com | 701998.com | www.050448.com | www.sf1.com | www.034787.com | www.379162.com | www.904027.com | www.686298.com | www.067210.com | www.95160.cc | www.53tf.com | www.994575.com | www.278123.com | www.4772.top | www.7478.pw | www.719570.com | www.55es.com | www.82zh.com | 大赢家彩票平台www.371679.com | 886874.com | www.661176.com | www.615375.com | www.388479.com | 4368.biz | www.15701.com | www.758399.com | www.40qp.com | www.099510.com | www.997.date | www.21396.cc | www.9747.cc | www.60155.cc | www.155216.com | www.0728.tv | www.977526.com | www.503592.com | www.228282.com | www.pc.com | 072628.com | 019963.com--7622.com | www.52723.com | www.61vo.com | 500彩票www.50026b.com | www.227530.com | 034546.com | www.703083.com | 大赢家彩票网www.178293.com | 974461.com | www.984015.com | www.966341.com | www.974208.com | 012773.com | www.865376.com | www.329461.com | 476934.com | 081057.com | www.552944.com | www.87111.com | www.mn48.com | www.857963.com | www.331250.com | www.652583.com | www.aq17.com | www.679507.com | www.70044.com | www.604418.com | 539207.com | 55803.com | 049118.com | www.819333.com | www.935196.com | www.542038.com | www.580127.com | www.f65.cn | www.490225.com | www.22425.com | 709437.com | www.004232.com | www.294618.com | www.71958.com | 554126.com | www.309298.com | www.983540.com | www.462123.com | www.882720.com | www.590330.com | www.581838.com | www.547361.com | www.829439.com | www.415.bid | www.815292.com | www.34ub.com | www.595288.com | www.vm98.com | www.745612.com | www.30968.com | www.508798.com | www.6133.cm | 983484.com | www.625385.com | www.610131.com | www.22310.com | www.9091.top | www.fd04.com | 984364.com | www.954857.com | www.989823.com | www.23998.com | www.024851.com | www.36466.cc | www.843232.com | www.324965.com | 756176.com | www.tz56.com | 500彩票www.51515x.com | 82992.com | www.501441.com | www.92633.com | 幸运彩票www.666937.com | www.58nt.com | www.671111.com | www.1oo.com | www.434637.com | www.123859.com | www.862146.com | www.577580.com | www.090328.com | 399677.cc | www.050015.com | 122364.com | www.090790.com | www.947387.com | www.127909.com | www.102964.com | www.91315.com | 216414.com | www.073407.com | www.6585.in | 好彩头彩票www.23579f.com | www.802072.com | www.244545.com | www.094104.com | www.629677.com | www.p74.com | www.481738.com | 048843.com | www.486234.com | www.62161.cc | 亚洲彩www.68568s.com | www.3831.biz | www.744898.com | www.7510.cn | www.638494.com | www.022545.com | www.8323.loan | www.75593.cc | www.cz84.com | 883469.com | www.974616.com | www.811515.com | www.380969.com | www.479777.com | www.292378.com | 爱米彩www.am1115.com | www.215799.com | 985483.com | www.139917.com | 948826.com | www.65929.com | www.789629.com | www.96698.com | www.hj59.com | www.789430.com | www.365771.com | www.178848.com | www.k26.website | www.486097.com | PK彩票www.8499r.com | www.417920.com | 550966.com | www.908938.com | www.1921.blue | www.988735.com | 99彩票www.062766.com | 487744.com | www.810698.com | 480736.com | www.7569.vip | 990873.com | www.792363.com | 331093.com | www.814827.com | www.290059.com | www.44gg.cc | www.475660.com | www.966601.com | www.860595.com | www.063622.com | www.447587.com | www.913892.com | www.341610.com | www.291376.com | www.84xi.com | 326106.com | www.699365.cc | www.527090.com | www.25345.com | www.31138.com | www.355176.com | www.624533.com | www.146062.com | www.646296.com | www.700484.com | www.330848.com | www.880749.com | www.337625.com | www.598278.com | www.261161.com | 029625.com | www.451268.com | 大赢家彩票平台www.375963.com | 462282.com | www.879466.com | 845474.com | 500彩票www.557031.com | 七彩www.53900q.com | www.995048.com | www.365736.cc | www.031203.com | www.vf14.com | www.8220.top | www.7374.pw | www.672023.com | www.th16.com | www.361755.com | www.wn15.com | www.504709.com | www.217250.com | www.088171.com | 196577.com | www.736262.com | www.043669.com | www.77669.cc | www.080882.com | www.mk73.com | www.952075.com | www.336596.com | www.02942.com | www.105603.com | 076205.com | www.220341.com | 52489.cc | www.232753.com | www.676903.com | www.882680.com | www.528238.com | www.035116.com | www.7768.org | 70993.com | www.776832.com | gf02.com | www.05750.cc | x18.top | www.041314.com | cp9708.com | www.365833.com | www.gw14.com | www.570448.com | www.84.cc | www.598727.com | www.cx51.com | www.640802.com | www.828708.com | www.248220.com | www.2255.date | 爱购彩票www.483552.com | www.271455.com | 898143.com | www.225370.com | www.739245.com | www.318959.com | 114902.com | www.31953.com | 059895.com | www.088327.com | www.176916.com | 438506.com | www.126482.com | www.626692.com | www.596882.com | 78jc.com | www.397226.com | www.302686.com | www.075919.com | www.tt8.cc | 557630.com | www.699869.com | www.696963.com | www.077928.com | www.44205.com | www.76em.com | www.ao32.com | 彩客博www.8667k.com | 915116.com | www.560893.com | www.644390.com | www.358898.com | www.025526.com | www.653759.com | www.0665.vip | www.935783.com | 425005.com | www.344598.com | www.239827.com | www.00rfd.com | www.315005.com | 125286.com | www.306566.com | www.cai2666.com | www.32150.cc | 106705.com | 570223.com | www.397701.com | www.153231.com | www.05jg.com | 32mj.com | www.411664.com | www.083957.com | www.ao7.cc | 81927.com | www.148944.com | 386176.com | www.184893.com | 彩多多www.78949p.com | www.196888.com | 577390.com | www.72872.cc | www.122976.com | www.0850.cc | www.139893.com | 820621.com | 554016.com | www.285739.com | www.hp51.com | www.386887.com | 654710.com | www.486477.com | www.22972.com | 501525.com | www.852534.com | www.569308.com | www.097368.com | www.44ej.com | www.000329.com | www.zm40.com | 111472.com | www.673418.com | www.015949.com | www.54544.cc | 68彩票www.68689q.com | www.588505.com | www.411473.com | www.101937.com | www.sl15.com | 949547.com | 646123.com | www.256382.com | www.169134.com | www.954116.com | www.037709.com | 192564.com | www.515468.com | www.05611.com | www.157892.com | www.170712.com | 036593.com | www.19588.com | www.648966.com | www.609048.com | 凤凰彩票www.5091l.com | www.862620.com | www.828254.com | www.360981.com | www.079400.com | 大赢家彩票平台www.178352.com | 336193.com | www.028961.com | 好运彩吧www.030238.com | www.890241.com | www.42ja.com | www.573480.cc | www.61250.com | 898745.com | www.487643.com | www.15546.com | www.046172.com | www.45oh.com | 586857.com | www.659103.com | www.031038.com | www.jy4.com | 994348.com | www.710029.com | 乐购彩www.lg36.com | www.158726.com | www.381477.com | www.006419.com | www.3326.in | www.lw48.com | www.694856.com | www.31722.cc | www.51fm.com | www.402983.com | www.662644.com | www.327186.com | www.2795.biz | www.xf8.com | 408477.com | www.675283.com | www.685883.com | www.36536.cc | www.636644.com | www.342533.com | www.6521.biz | 599292.com--50.cc | www.288683.com | www.jz09.com | www.948954.com | www.153223.com | www.63012.com | www.35ve.com | 54886.com | www.751270.com | www.220303.com | www.999227.com | www.29003.cc | www.626008.com | www.374244.com | www.82851.com | www.37hc.com | 中彩网www.61233j.com | 842234.com | www.660262.com | 724433.com | www.570113.com | www.19168.com | 中国福利彩票www.3478i.cc | www.699653.com | www.557326.com | www.247794.com | www.335023.com | www.79xp.com | www.881054.com | 449116.com | www.700982.com | www.101408.com | www.cai1238.com | 8号彩票www.81520s.com | 彩82www.c5128.com | www.174938.com | www.129048.com | www.mz64.com | gx26.com | www.588371.com | www.613315.com | www.414683.com | www.320063.com | www.38wc.com | www.867630.com | www.194614.com | www.1754.vip | 027635.com | www.137912.com | www.15033.com | 639689.com | www.676608.com | www.227629.com | www.031979.com | www.0631.bid | 034995.com | www.262597.com | www.33338.com | www.369081.com | www.31707.com | www.677291.com | www.738339.com | www.565802.com | www.29857.com | www.nq88.com | www.971353.com | 吉利彩票www.80075q.com | www.501951.com | www.h24.xyz | www.741239.com | www.002205.com |